This breakthrough was made possible by the development of a novel source of
attosecond pulses.
In the hope that this analysis can become even more exact, the laser physicists from the Laboratory
of Attosecond Physics at Ludwig - Maximilians - Universitaet (LMU) in Munich and the Max Planck Institute for Quantum Optics have developed an infrared light source that has an enormously broad spectrum of wavelengths.
Now, a team headed by Dr. Peter Baum and Prof. Ferenc Krausz from the Laboratory for
Attosecond Physics (LAP), LMU and the Max - Planck Institute of Quantum Optics (MPQ) has succeeded in developing a new technique for controlling ultrafast electron pulses.
Their main objective is to learn to recognise how the structure of molecules changes
with attosecond time resolution.
Physicists at the Laboratory
for Attosecond Physics (LAP), a joint venture between the Ludwig - Maximilians - Universität Munich (LMU) and the Max Planck Institute of Quantum Optics (MPQ), have now succeeded in meeting the conditions necessary to achieve this goal.
This interaction takes place
in attosecond times (i.e. billionths of a billionth of a second).
We do not know all the details,» says Johan Mauritsson, researcher in the field of
attosecond science at Lund University in Sweden.
These pulses can be used to follow the motion of electrons within the inner shells of atoms in real time by freezing this motion
at attosecond shutter speeds.
Today scientists generally use argon gas as the medium for generating
attosecond laser pulses with HHG.
Electron pulses with durations in the femtosecond to
attosecond range (10-15-10-18 s) would be ideal for monitoring processes inside matter with the required resolution in both space and time, i.e. in four dimensions.
No research group has previously succeeded in
generating attosecond pulses with the required photon density in this spectral region.
The authors of the study, experimentalists led by Prof. Dr. Hans Jakob Wörner from the Swiss Federal Institute of Technology (ETH Zurich) and theoreticians from Russia, Denmark, Belgium and Canada, including Oleg Tolstikhin from MIPT, are investigating what is known as «attophysics» - the study of events with
attosecond time resolution, i.e. a billionth of a billionth of a second (10 ^ -18 of a second).
«Ultrafast electron oscillation and dephasing monitored by
attosecond light source: Petahertz electron oscillation observed using chromium doped sapphire solid - state material.»
With this novel tool at hand, the researchers flashed krypton atoms with
optical attosecond pulses.
Control of light with
attosecond resolution opens fascinating views on electron dynamics on the atomic scale.
Their next goal is to generate single
attosecond electron wave packets, in order to follow what happens during subatomic interactions with even higher precision.
Schultze et al. applied
attosecond spectroscopy to glimpse this motion in a sample of silicon, the semiconducting building block of modern integrated circuits (see the Perspective by Spielmann).
A pulse of visible light just 380
attoseconds long served as a flashbulb to probe how electrons emit photons when struck with light
«The detailed dynamics resulting from these interactions raise many questions, which we can now address experimentally using our new
attosecond source.»
Last year, the team created brief pulses of visible light too, each
380 attoseconds long.
«Race of the electrons: Laser pulses can be used to track the motion of electrons in metals with
attosecond precision.»
Dr. Hiroki Mashiko, a NTT scientist of the team, said, «We contrived the robust pump - probe system with an extremely short
isolated attosecond pulse, which led to the observation of the fastest electron oscillation in solid - state material in recorded history.
Our lasers are helping scientists to break new ground in many applications ranging
from attosecond physics to forensics and genomics.
Physicist Ferenc Krausz, who led the project, plans to go further: «We believe that we should get down to 100
attoseconds by the end of the year.»
Their mercurial movements can be over in
just attoseconds — billionths of a billionth of a second — yet they drive our electronic devices, every chemical reaction in nature and every thought in our heads.
Monti's «stopwatch» makes it possible to track moving electrons at a resolution of a
mere attosecond — a billionth of a billionth of a second.
The reported advances in understanding photoemission from solids became feasible based on recently
developed attosecond laser techniques.
Electron ejection from multiple N2 orbitals, controlled by the molecule's orientation relative to a laser,
produces attosecond light spectra that can reveal molecular dynamics.
In addition, the researchers were also able to determine, for the first time, how the energy of the incident photon is quantum mechanically distributed between the two electrons of the helium atom in the final
few attoseconds before the emission of one of the particles.
To comprehend how brief that is, consider that one second contains about twice as
many attoseconds as there are seconds in the 14 - billion - year life of the universe, says physicist Johan Mauritsson of Lund University in Sweden, who led the study.
The Centre is the only place in the country to have the machine in its
Australian Attosecond Science Facility.
In previous
attosecond experiments, it has only been possible to observe the interaction of inner shell electrons with a single XUV photon.
In this image, patterns captured at
attosecond intervals have been superimposed, thus revealing, in real time, the kind of electron motions that underlie atomic and subatomic phenomena.
This hardly conceivable resolution allows timing the race of electrons in experiments that were performed at Bielefeld University using
advanced attosecond time - resolved laser spectroscopy.
That way, the team succeeded in
creating attosecond pulse radiation a hundred times more intense than simple sine - shaped waves could produce.
There is a temporal realm called the Planck scale, where
even attoseconds drag by like eons.
The frequency of the lightwave - field in the visible and ultraviolet region can reach the petahertz (PHz: 1015 of a hertz), which means that the oscillation periodicity can
achieve attosecond (as: 10 - 18 of a second) duration.
We implemented self -
referenced attosecond photoelectron interferometry to measure the temporal profile of the forward and backward electron wave packets emitted upon photoionization of camphor by circularly polarized laser pulses.
The scientists beamed light flashes lasting only a few hundred
attoseconds onto 50 nanometer thick glass particles, which released electrons inside the material.
Of course, one day, perhaps not so very far in the future, even the
speedy attosecond will fail to satisfy.
In the next step, the physicists plan an experiment in which they will time resolve the interaction by splitting the high -
intensity attosecond pulse into separate pump and probe pulses.
In a first series of experiments, the high -
energy attosecond pulses were focused on a stream of xenon gas.
These light pulses with different wavelengths, whose time separation can be adjusted with
attosecond accuracy, are very powerful tools to investigate the structure of matter and the dynamics of ultrafast physical processes and chemical reactions.