Atmospheric concentrations
of organic aerosol are frequently similar to those of industrial sulphate aerosol.
Knowledge on the hygroscopicity of OA and measurements of optical properties
of the organic aerosol constituents are summarized.
The ensemble of the simulations was used to build an integrated and robust view of our understanding
of organic aerosol sources and sinks in the troposphere.
Her research experience includes modeling
of organic aerosol oxidation at LBNL, fabrication and optimization of high performance semiconductor nanoparticle - based image sensors as Manager of Materials Development at InVisage Technologies, Inc., and foundational and applied research as a Research Staff Member at IBM's Almaden Research Center on transformations in dielectrics, semiconductors, metals, and polymer films.
Volatility is a key property
of organic aerosol because it determines the partitioning between the gas and particle phases, and thus the formation of SOA particles.
Along the PlaetSolar itinerary, the colored dots represent the concentration
of organic aerosols, from blue (light concentration) to red (strong concentration).
However, to make climate models more accurate, we are focused on developing a better understanding of the dynamics
of organic aerosols formed from plant - based organic vapors and their interaction with aerosols emitted from human activities,» said Dr. Chen Song, a PNNL atmospheric scientist.
Why It Matters: Current atmospheric computer models do not consider the evolving chemistry
of the organic aerosols.
The researchers at PNNL and UCI are continuing to answer questions about the properties
of organic aerosols in the atmosphere.
International research group shows that the aging
of organic aerosols is caused by OH radicals
The experiments showed that the mass and composition
of organic aerosols are significantly influenced by OH radicals.
The absorbing effect
of organic aerosols is thus implicitly included in the BC estimate, although to an unknown extent.
Chamber research is focused on understanding the lifecycle
of organic aerosols, including their formation, growth, aging (oxidation), re-volatilization, and effect on cloud formation.
Topics that I work on or plan to work in the future include studies of: + missing aerosol species and sources, such as the primary oceanic aerosols and their importance on the remote marine atmosphere, the in - cloud and aerosol water aqueous formation
of organic aerosols that can lead to brown carbon formation, the primary terrestrial biological particles, and the organic nitrogen + missing aerosol parameterizations, such as the effect of aerosol mixing on cloud condensation nuclei and aerosol absorption, the semi-volatility of primary organic aerosols, the importance of in - canopy processes on natural terrestrial aerosol and aerosol precursor sources, and the mineral dust iron solubility and bioavailability + the change of aerosol burden and its spatiotemporal distribution, especially with regard to its role and importance on gas - phase chemistry via photolysis rates changes and heterogeneous reactions in the atmosphere, as well as their effect on key gas - phase species like ozone + the physical and optical properties of aerosols, which affect aerosol transport, lifetime, and light scattering and absorption, with the latter being very sensitive to the vertical distribution of absorbing aerosols + aerosol - cloud interactions, which include cloud activation, the aerosol indirect effect and the impact of clouds on aerosol removal + changes on climate and feedbacks related with all these topics In order to understand the climate system as a whole, improve the aerosol representation in the GISS ModelE2 and contribute to future IPCC climate change assessments and CMIP activities, I am also interested in understanding the importance of natural and anthropogenic aerosol changes in the atmosphere on the terrestrial biosphere, the ocean and climate.
Not exact matches
She decided to study the role that
organic particles play in cloud droplet formation, because a large proportion
of marine
aerosols — which have a significant climate impact — are
organics.
The results imply that the interaction between
organic and sulfuric acids promotes efficient formation
of organic and sulfate
aerosols in the polluted atmosphere because
of emissions from burning
of fossil fuels, which strongly affect human health and global climate.
Carbonaceous PM is made up
of black carbon, primary
organic aerosol (POA) and, especially, secondary
organic aerosol (SOA), which is known to contain harmful reactive oxygen species and can damage lung tissue.
Aerosol nucleation is known to require sulphuric acid, but Kirkby's team found that it is not enough by itself at low altitudes — the presence
of an additional
organic trace vapour is needed (Nature, DOI: 10.1038 / nature10343).
They also play a role in the formation
of secondary
organic aerosols — air pollutants produced when sunlight,
organic molecules and airborne chemicals come together and interact.
Xiao used battery powered
aerosol monitors to measure indoor concentrations
of fine particulate matter, or particles 2.5 micrometers in diameter or smaller, which consists mainly
of black carbon and
organic carbon.
Such model included meteorological factors like levels
of aerosols, anthropogenic and biogenic volatile
organic compounds (VOCs), ozone, carbon dioxide, methane, and other items that influence global temperature — the surface albedo among them.
It involves generating
aerosol droplets that consist
of a solid core and a shell made
of organic materials that mimic some
of the polymers one would find in electronics.
Forest fires in the lower latitudes, however, are actually beneficial sources
of black carbon because it is coupled with
organic aerosols and ends up reflecting light and heat, causing the surrounding area to cool.
This provides a new insight into the conventional belief that tree leaves are the primary source
of organic gases and
aerosols which can affect the cloud formation.
Yet, the factors that influence the formation
of these
aerosols, known as secondary
organic aerosol or SOA, are often assumed.
A study published April 7 in PNAS Online Early Edition describes how a team
of scientists, including researchers from the University
of California, Davis, showed that vapor losses to the walls
of laboratory chambers can suppress the formation
of secondary
organic aerosol, which in turn has contributed to the underprediction
of SOA in climate and air quality models.
In one
of the first studies
of its kind, scientists have found that tar sands production in Canada is one
of North America's largest sources
of secondary
organic aerosols — air pollutants that affect the climate, cloud formation and public health.
Laboratory chamber walls have been stealing vapors, causing researchers to underestimate the formation
of secondary
organic aerosol in the atmosphere.
The resulting mass concentration
of secondary
organic aerosols was roughly between five and 100 μg / m3.
It drives the formation
of much
of the atmospheric
organic aerosol present in our environment.
The new findings help to explain a significant part
of the
organic mass
of aerosol particles in the air, which had remained mysterious to the scientists so far.
«The results suggest that about 10 percent
of the reacting VOC mass is converted tosecondary
organic aerosol over the tree tops.
This includes the role
of oxidized volatile
organic compounds, such as limonene and alpha - pinene, the typical scents
of the citrus fruits and coniferous forests, in
aerosol formation.
Using aircraft to measure air pollution over the Alberta tar sands region, the researchers found that tar sands production emitted between 55 and 101 metric tonnes
of secondary
organic aerosols per day.
In research recently published in Environmental Science & Technology, Waring describes the role
of limonene, the
organic compound that gives cleaners and air fresheners an orange scent and acts as a solvent, in the formation
of secondary
organic aerosols.
By adjusting elements
of the test, such as the air exchange rate, which is the number
of times per hour indoor air is replaced by outdoor air, as well as the concentrations
of terpene and ozone in the chamber, the group was able to ascertain how those variables each affected the formation
of secondary
organic aerosols.
The cooling effect
of aerosols can partly offset global warming on a short - term basis, but many are made
of organic material that comes from sources that scientists don't fully understand, said Joost de Gouw, a research physicist at NOAA's Earth System Research Laboratory in Boulder, Colo., who is unaffiliated with the studies.
And while researchers are still striving to fully understand the health and environmental impact
of increased levels
of secondary
organic aerosols in the atmosphere, studies have linked exposure to outdoor
aerosols generally to morbidity and mortality outcomes.
With 18 different scenarios tested, the team calculated a range
of peak formation
of secondary
organic aerosols when typical concentrations
of limonene were introduced to ozone - rich environments with a range
of air exchange rates.
Shiraiwa, M., Pfrang, C., Koop, T., and Pöschl, U.: Kinetic multilayer model
of gas - particle interactions in
aerosols and clouds (KM - GAP): linking condensation, evaporation and chemical reactions
of organics, oxidants and water, Atmospheric Chemistry and Physics, 12, 2777 - 2794, 2012.
The specialized instruments onboard the aircraft sampled the plume for
aerosol particle size distribution and composition as well as concentrations
of pollutant gases such as sulfur dioxide, nitric oxide, nitrogen dioxide, ozone, and volatile
organic compounds (VOCs).
Shiraiwa, M., Ammann, M., Koop, T., and Pöschl, U: Gas uptake and chemical aging
of semi-solid
organic aerosol particles, Proceedings
of the National Academy
of Sciences, 108, 11003 - 11008, 2011.
«Photolytic processing
of secondary
organic aerosols dissolved in cloud droplets.»
Berkemeier, T., S.S. Steimer, U. K. Krieger, T. Peter, U. Pöschl, M. Ammann, and M. Shiraiwa: Ozone uptake on glassy, semi-solid and liquid
organic matter and the role
of reactive oxygen intermediates in atmospheric
aerosol chemistry, Physical Chemistry Chemical Physics 18 (18), 12662 - 12674, 2016.
«Nighttime chemical evolution
of aerosol and trace gases in a power plant plume: Implications for secondary
organic nitrate and organosulfate
aerosol formation, NO3 radical chemistry, and N2O5 heterogeneous hydrolysis.»
New study shows the molecular details
of how
organic aerosol helps heat up and color the haze over megacities
Song and fellow researchers published research in 2007 that addressed assumptions in the ability
of diesel exhaust
organic aerosols to mix with
organic aerosols from tree evaporate.
On high biomass burning days, both biomass burning and human - based activities equally contributed to levels
of secondary
organic aerosol downwind
of Mexico City.
The largest portion
of these submicron
aerosols is
organic, or carbon - containing, and is classified as two kinds: primary and secondary.
Methods: In a series
of experiments, the team synthesized
organic aerosols.