Effects of anthropogenic emissions
on aerosol formation from isoprene and monoterpenes in the southeastern United States
Whether these reactions produce condensing vapours that can condense onto the smallest particles or even molecules can have strong impacts
on aerosol formation.
Not exact matches
The
aerosols catalyze the
formation of ice in the clouds, which could increase precipitation, although more research needs to be done
on that linkage, Creamean said.
Despite its smaller ash cloud, El Chichn emitted more than 40 times the volume of sulfur - rich gases produced by Mt. St. Helens, which revealed that the
formation of atmospheric sulfur
aerosols has a more substantial effect
on global temperatures than simply the volume of ash produced during an eruption.
At least over the oceans, the pre-industrial cloud conditions would have been considerably different from those of today; this implies that the
aerosols we have been adding to the atmosphere may have had a significant effect
on global patterns of cloud
formation and rain.
Also facing elimination are the Orbiting Carbon Observatory 3, which would observe carbon dioxide flows; a mission to the space station that would have supported tests of a spectrometer intended to measure solar reflection; and Plankton,
Aerosol, Cloud, ocean Ecosystem, a satellite that would measure the colors of the ocean to gauge the global flow of algae and the influence of ocean
aerosols on cloud
formation.
«Huge amounts of
aerosols from Asia go as high as six miles up in the atmosphere and these have an unmistakable impact
on cloud
formations and weather.»
«We're not clear yet
on what components of these emissions are the biggest contributors to ozone
formation or
aerosol formation,» says Coggon, «so that's what we'll be trying to figure out.»
They found that galactic cosmic rays exert only a small influence
on the
formation of sulphuric acid — dimethylamine clusters (the embryonic stage before
aerosols may act as cloud condensation nuclei).
However, I am not optimistic — the specifics of the small scale physics (
aerosol indirect effects
on clouds, sea ice
formation, soil hydrology etc.) are so heterogeneous that I don't see how you can do without calculating the details.
Solar activity impacts
on climate are a fascinating topic, and encompass direct radiative processes, indirect effects via atmospheric chemistry and (potentially)
aerosol formation effects.
The results presented are of the impact of ionization
on the
formation rate of
aerosols with size ~ 4 nanometers (nm), as shown in the figure below:
Perhaps the thresholds for a CRF - cloud correlation was higher then than it has been for the past 40 years (one might imagine that in periods where the air is rather clear of man made
aerosols, the threshold for CRF effects
on cloud
formation become higher... and so
on).
Yes, there are physical mechanisms to connect GCM's to
aerosol formation — however, GCM's aren't the only forcing
on the system.
This paper re-states the grand Svensmark theory and attempts to address the work that has shown cosmic rays can not be a significant influence
on climate because most
aerosols run out of stuff to become big enough for cloud
formation.
This section only assesses the aspects that are unique to the aviation sector, namely the
formation of persistent condensation trails (contrails), their impact
on cirrus cloudiness, and the effects of aviation
aerosols.
In summary the findings to date indicate that the effect of cosmic rays
on cloud
formation is small compared to the large variations in natural biogenic
aerosol emissions.
Effect of pellet boiler exhaust
on secondary organic
aerosol formation from α - pinene.
Here, we report unique observations
on atmospheric
aerosol formation based
on measurements at the SMEAR II station, Finland, over a solar cycle (years 1996 — 2008) that shed new light
on these presumed relationships.
A short while ago, Eli posted about Finnish research
on the
formation of small atmospheric
aerosols.
46 Based
on surface
aerosol measurements at one site, Kulmala et al. (2010) found no connection between GCR 47 and new particle
formation or any other
aerosol property over a solar cycle (1996 — 2008).
Joe Ceonnia: ``... it seems to me as if this program is all over the globe» Joe, by observing the astoundingly unnatural patterns of atmospheric
aerosols on cloud
formations around the planet — via NASA Worldview (online)-- one can visibly observe the effects of geoengineering around the world.
Romakkaniemi, S., Maalick, Z., Hellsten, A., Ruuskanen, A., Väisänen, O., Ahmad, I., Tonttila, J., Mikkonen, S., Komppula, M., and Kühn, T.:
Aerosol — landscape — cloud interaction: signatures of topography effect
on cloud droplet
formation, Atmos.
New information from dedicated recent and future field campaigns is expected to shed light
on organic
aerosol formation processes and how they are altered in the presence of anthropogenic pollution.
If a cloud doesn't form then because of lack of
aerosols to start
formation, chill that sucker down some more to form ice crystals and it should make its
on substrate to form.
The 2014 Biogenic
Aerosols — Effects
on Clouds and Climate (BAECC) field campaign in Finland has provided rich data
on processes related to
aerosol, cloud, and snow
formation.
The current focus of the program is
aerosol radiative forcing of climate:
aerosol formation and evolution and
aerosol properties that affect direct and indirect influences
on climate and climate change.»
With cloud tops warmer than -38 degrees Celsius, ice
formation depends
on aerosols that preferentially freeze at warm temperatures, referred to as ice nuclei.
The Indirect and Semi-Direct
Aerosol Campaign (ISDAC) field campaign, deployed from Barrow, Alaska,
on a Canadian National Research Council Convair - 580 jet in April 2008, provided improved observations of two new cases of single - layer, mixed - phase, stratiform clouds that are well - suited to test our understanding of ice
formation.
These clouds then glaciate in higher levels, which could result in either more or less vigorous precipitation
formation depending
on the background
aerosol levels and atmospheric stability (Khain et al., 2004).
On the other hand, if some of the anthropogenic
aerosols act as ice nuclei, supercooled clouds could be converted into ice clouds by the glaciation indirect effect (Lohmann, 2002), resulting in more efficient precipitation
formation.
It has been hypothesized that galactic cosmic rays (GCR) create atmospheric ions which facilitates
aerosol nucleation and new particle
formation with a further impact
on the cloud
formation (Kazil et al., 2012; Pierce and Adams, 2009).
Based
on surface
aerosol measurements at one site, Kulmala et al. (2010) found no connection between GCRand new particle
formation or any other
aerosol property over a solar cycle (1996 — 2008).
In the article «Global atmospheric particle
formation from CERN CLOUD measurements,» sciencemag.org, 49 authors concluded «Atmospheric
aerosol nucleation has been studied for over 20 years, but the difficulty of performing laboratory nucleation - rate measurements close to atmospheric conditions means that global model simulations have not been directly based
on experimental data.....
Under strict temperature and humidity conditions, investigations in this laboratory provide new information
on the particular
aerosol particles that can lead to the
formation of these clouds.
In addition to the complex physics of fog
formation and transport, recent research suggests that microscopic
aerosol particles may be critical players in fog dynamics and its effect
on coastal human and ecological systems.
Chamber research is focused
on understanding the lifecycle of organic
aerosols, including their
formation, growth, aging (oxidation), re-volatilization, and effect
on cloud
formation.
Heterogeneous ice nucleation
on atmospheric
aerosols: a review of results from laboratory experiments / C. Hoose & O. Mohler Institute for Meteorology and Climate Research — Atmospheric
Aerosol Research, Karlsruhe Institute of Technology, Karlsruhe, Germany / Published: 29 October 2012 Abstract: A small subset of the atmospheric aerosol population has the ability to induce ice formation at conditions under which ice would not form without them (heteroge - neous ice nucle
Aerosol Research, Karlsruhe Institute of Technology, Karlsruhe, Germany / Published: 29 October 2012 Abstract: A small subset of the atmospheric
aerosol population has the ability to induce ice formation at conditions under which ice would not form without them (heteroge - neous ice nucle
aerosol population has the ability to induce ice
formation at conditions under which ice would not form without them (heteroge - neous ice nucleation).
Here, in part I, I'll review some of the basic processes that are important in determining the climate effects of
aerosols, focusing in particular
on their
formation.
The present 3 - D modeling study focuses
on aerosol chemical composition change since preindustrial times considering the secondary organic
aerosol formation together with all other main
aerosol components including nitrate.
Timonen, H., Karjalainen, P., Saukko, E., Saarikoski, S., Aakko - Saksa, P., Simonen, P., Murtonen, T., Dal Maso, M., Kuuluvainen, H., Bloss, M., Ahlberg, E., Svenningsson, B., Pagels, J., Brune, W. H., Keskinen, J., Worsnop, D. R., Hillamo, R., and Rönkkö, T.: Influence of fuel ethanol content
on primary emissions and secondary
aerosol formation potential for a modern flex - fuel gasoline vehicle, Atmos.
The climate feedbacks involved with these changes, which are key in understanding the climate system as a whole, include: + the importance of
aerosol absorption
on climate + the impact of
aerosol deposition which affects biology and, hence, emissions of
aerosols and
aerosol precursors via organic nitrogen, organic phosphorus and iron fertilization + the importance of land use and land use changes
on natural and anthropogenic
aerosol sources + the SOA sources and impact
on climate, with special attention
on the impact human activities have
on natural SOA
formation In order to quantitatively answer such questions I perform simulations of the past, present and future atmospheres, and make comparisons with measurements and remote sensing data, all of which help understand, evaluate and improve the model's parameterizations and performance, and our understanding of the Earth system.
BAECC was designed to obtain important details
on processes related to
aerosol, cloud, and snow
formation that are not currently well understood or well represented in earth system models.
Topics that I work
on or plan to work in the future include studies of: + missing
aerosol species and sources, such as the primary oceanic
aerosols and their importance
on the remote marine atmosphere, the in - cloud and
aerosol water aqueous
formation of organic
aerosols that can lead to brown carbon
formation, the primary terrestrial biological particles, and the organic nitrogen + missing
aerosol parameterizations, such as the effect of
aerosol mixing
on cloud condensation nuclei and
aerosol absorption, the semi-volatility of primary organic
aerosols, the importance of in - canopy processes
on natural terrestrial
aerosol and
aerosol precursor sources, and the mineral dust iron solubility and bioavailability + the change of
aerosol burden and its spatiotemporal distribution, especially with regard to its role and importance
on gas - phase chemistry via photolysis rates changes and heterogeneous reactions in the atmosphere, as well as their effect
on key gas - phase species like ozone + the physical and optical properties of
aerosols, which affect
aerosol transport, lifetime, and light scattering and absorption, with the latter being very sensitive to the vertical distribution of absorbing
aerosols +
aerosol - cloud interactions, which include cloud activation, the
aerosol indirect effect and the impact of clouds
on aerosol removal + changes
on climate and feedbacks related with all these topics In order to understand the climate system as a whole, improve the
aerosol representation in the GISS ModelE2 and contribute to future IPCC climate change assessments and CMIP activities, I am also interested in understanding the importance of natural and anthropogenic
aerosol changes in the atmosphere
on the terrestrial biosphere, the ocean and climate.