Many of the modelling studies performed since the TAR have investigated the RF of
organic carbon aerosols from both fossil fuel and biomass burning aerosols, and the combined RF of both components.
· The study found evidence to link brown carbon — a form of
organic carbon aerosols — to warming.
Photo credit: DRIChakrabarty and colleagues found to their surprise that funeral pyre emissions contain sunlight - absorbing
organic carbon aerosols known as brown carbon.
Spracklen, D. V., J. A. Logan, L. J. Mickley, R. J. Park, R. Yevich, A. L. Westerling, and D. A. Jaffe, 2007: Wildfires drive interannual variability of
organic carbon aerosol in the western US in summer.
Wildfires drive interannual variability of
organic carbon aerosol in the western US in summer
The response of biogenic secondary
organic carbon aerosol production to a temperature change, however, could be considerably lower than the response of biogenic VOC emissions since aerosol yields can decrease with increasing temperature.
Historical emissions of black and
organic carbon aerosol from energy - related combustion, 1850 — 2000.
However, coatings of
organic carbon aerosol on hygroscopic aerosol such as sulphate may lead to suppression of the rate of water uptake during cloud activation (Xiong et al., 1998; Chuang, 2003).
Not exact matches
Carbonaceous PM is made up of black
carbon, primary
organic aerosol (POA) and, especially, secondary
organic aerosol (SOA), which is known to contain harmful reactive oxygen species and can damage lung tissue.
Xiao used battery powered
aerosol monitors to measure indoor concentrations of fine particulate matter, or particles 2.5 micrometers in diameter or smaller, which consists mainly of black
carbon and
organic carbon.
Such model included meteorological factors like levels of
aerosols, anthropogenic and biogenic volatile
organic compounds (VOCs), ozone,
carbon dioxide, methane, and other items that influence global temperature — the surface albedo among them.
Forest fires in the lower latitudes, however, are actually beneficial sources of black
carbon because it is coupled with
organic aerosols and ends up reflecting light and heat, causing the surrounding area to cool.
The team evaluated simulated cloud fields from the multi-scale
aerosol - climate model and examined how specific human - caused
aerosols, such as sulfate, black
carbon (soot), and
organic carbon affect those clouds and, in turn, the climate.
The team injected citric, adipic, and fulvic acid into the chamber as seed
aerosols, and then introduced a secondary
organic aerosol from α - pinene, a
carbon - containing compound derived from pine trees.
The largest portion of these submicron
aerosols is
organic, or
carbon - containing, and is classified as two kinds: primary and secondary.
The PNNL study measured how, in the atmosphere, these
aerosols interact with and mix with other volatile or semi-volatile
organic compounds, the
carbon - centric chemicals that evaporate from both natural and human - made sources.
Results: Today's climate models regard
organic aerosols as static
carbon - based molecules, but scientists at Pacific Northwest National Laboratory and the University of California, Irvine showed that the particles are very dynamic.
These have garnered more than 600 citations advancing our understanding of what the research field calls secondary
organic aerosols — or SOA for short — and how the
carbon - containing
aerosol particles mix in the atmosphere.
The CARES field campaign was designed to increase scientific knowledge about the evolution of black
carbon, primary
organic aerosols (POA), and secondary
organic aerosols (SOA) from both human - caused and natural (biogenic) sources.
c G: greenhouse gases; Sul: direct sulphate
aerosol effect; Suli: (first) indirect sulphate effect; OzT: tropospheric ozone; OzS: stratospheric ozone; Vol: volcanism; Sol: solar; BC+OM: black
carbon and
organic matter.).
Biomass burning is a big source of black
carbon and
organic aerosols (warming), CO and VOCs (ozone precursors), also SO2 (leading to sulphate
aerosols)(cooling).
The answer, of course, is that Pieter is talking about
carbon particles (
aerosols, often called black
carbon) and the post is talking about
carbon atoms in principally CO2, but also methane and
organic volatile moleclues.
Importantly, RCP4.5 considers the influence of sulfur
aerosols, as well as black and
organic carbon.
One notable change is the assimilation of
aerosol observations, including black and
organic carbon, sulfate and dust.
PACific Dust EXperiment «The long range transport of dust and anthropogenic
aerosols (e.g, black
carbon,
organics and sulfates, and air pollution from Eurasia, across the Pacific Ocean, into North America is one of the most wide spread and major pollution events on the planet.
BC FF is for black
carbon from fossil fuel and biofuel, POA FF is for primary
organic aerosol from fossil fuel and biofuel, BB is for biomass burning
aerosols and SOA is for secondary
organic aerosols.»
The brownish color of the cloud (which is visible when looking at the horizon) is due to absorption of solar radiation at short wavelengths (green, blue, and UV) by
organic and black
carbon aerosols as well as by NOx.
Black
carbon - Operationally defined
aerosol species based on measurement of light absorption and chemical reactivity and / or thermal stability; consists of soot, charcoal and / or possible light absorbing refractory
organic matter.
...
Aerosol species are grouped by the parameterization into three basic types: dust and metallic compounds, inorganic black
carbon, and insoluble
organic aerosols.
There is one aspect of climate change that is not fully established: the role of
aerosol pollution (aka global dimming) from mainly from sulfates and soot (black
carbon and
organic carbon).
Key
aerosol groups include sulfates,
organic carbon, black
carbon, nitrates, mineral dust, and sea salt.
However, the extent of black -
carbon - induced warming is dependent on the concentration of sulphate and
organic aerosols — which reflect solar radiation and cool the surface — and the origin of the black
carbon3, 4.
Cointegration indicates that internal climate variability and / or the omission of some components of radiative forcing (e.g., stratospheric water vapor, black or
organic carbon, nitrite
aerosols, etc.) do not impart a stochastic or deterministic trend that would interfere with the interpretation of temperature changes at the subdecadal scale (SI Appendix).
FIGURE 4 - 1 Annual mean
aerosol optical depth predicted by an
aerosol chemical transport model due to sulfate, mineral dust, sea salt, and
organic and black
carbon aerosols.
In general, primary
aerosol components (black
carbon, hydrocarbon - like
organic aerosol and biomass burning
organic aerosol) dominated the local traffic and wood burning emissions whereas secondary components (oxygenated
organic aerosol, nitrate, ammonium, and sulfate) dominated the PM1 chemical composition during the LRT episode.
Novakov, T., S. Menon, T.W. Kirchstetter, D. Koch, and J.E. Hansen, 2007: Reply to comment by R.L. Tanner and D.J. Eatough on «
Aerosol organic carbon to black
carbon ratios: Analysis of published data and implications for climate forcing».
First, we have to consider the effect of
aerosols, which start off as urban haze or rural smoke and ultimately become transcontinental and transoceanic plumes o ABCs consisting of sulfate, nitrate, hundreds of
organics, black
carbon, soil dust, fly ash, and other
aerosols.
In particular, we evaluate non-sea-salt sulfate (nss - SO4 =), ammonium (NH4 +), nitrate (NO3 --RRB-, black
carbon (BC), sea - salt, dust, primary and secondary
organics (POA and SOA) with a focus on the importance of secondary
organic aerosols.
Topics that I work on or plan to work in the future include studies of: + missing
aerosol species and sources, such as the primary oceanic
aerosols and their importance on the remote marine atmosphere, the in - cloud and
aerosol water aqueous formation of
organic aerosols that can lead to brown
carbon formation, the primary terrestrial biological particles, and the
organic nitrogen + missing
aerosol parameterizations, such as the effect of
aerosol mixing on cloud condensation nuclei and
aerosol absorption, the semi-volatility of primary
organic aerosols, the importance of in - canopy processes on natural terrestrial
aerosol and
aerosol precursor sources, and the mineral dust iron solubility and bioavailability + the change of
aerosol burden and its spatiotemporal distribution, especially with regard to its role and importance on gas - phase chemistry via photolysis rates changes and heterogeneous reactions in the atmosphere, as well as their effect on key gas - phase species like ozone + the physical and optical properties of
aerosols, which affect
aerosol transport, lifetime, and light scattering and absorption, with the latter being very sensitive to the vertical distribution of absorbing
aerosols +
aerosol - cloud interactions, which include cloud activation, the
aerosol indirect effect and the impact of clouds on
aerosol removal + changes on climate and feedbacks related with all these topics In order to understand the climate system as a whole, improve the
aerosol representation in the GISS ModelE2 and contribute to future IPCC climate change assessments and CMIP activities, I am also interested in understanding the importance of natural and anthropogenic
aerosol changes in the atmosphere on the terrestrial biosphere, the ocean and climate.
Theoretically, coatings of essentially non-absorbing components such as
organic carbon or sulphate on strongly absorbing core components such as black
carbon can increase the absorption of the composite
aerosol (e.g., Fuller et al., 1999; Jacobson, 2001a; Stier et al., 2006a), with results backed up by laboratory studies (e.g., Schnaiter et al., 2003).
However, sulphate is invariably internally and externally mixed to varying degrees with other compounds such as biomass burning
aerosol (e.g., Formenti et al., 2003), fossil fuel black
carbon (e.g., Russell and Heintzenberg, 2000),
organic carbon (Novakov et al., 1997; Brock et al., 2004), mineral dust (e.g., Huebert et al., 2003) and nitrate
aerosol (e.g., Schaap et al., 2004).