The problem with clouds in climate models are of two different types: the first is a microphysics / chemistry one, regarding the physics and chemistry of how a population of cloud particles interacts
with aerosol particles and evolves with time.
One of the key uncertainties is clouds, understanding the physics behind clouds and how clouds interact
with aerosol particles.
Shiraiwa, M., Sosedova, Y., Rouvière, A., Yang, H, Zhang, Y., Abbatt, J. P. D., Ammann, M., and Pöschl, U.: The role of longlived reactive oxygen intermediates in the reaction of ozone
with aerosol particles, Nature Chemistry, 3, 291 - 295, 2011.
In particular, they propose that cloud changes associated
with aerosol particles in the atmosphere could be causing the weekend effect, though other pollution processes can not be ruled out at this time.
Not exact matches
After allowing for humidity and rainfall, they found that «
aerosol optical thickness» — a measure of the concentration of atmospheric
particles — decreased by only 10 to 15 per cent compared
with the same periods in 2002 to 2007 (Geophysical Research Letters, in press).
During storms, they flew a research aircraft
with several powerful instruments, including one that can identify the type of
particle in a cloud and determine whether it was dust or some other type of
aerosol.
With PNNL's climate model, Smith created more than 1,400 potential scenarios to reflect the many possibilities surrounding
aerosols, tiny
particles including soot that float in the atmosphere.
It then combines
with pollutants from combustion — mainly nitrogen oxides and sulfates from vehicles, power plants and industrial processes — to create tiny solid
particles, or
aerosols, no more than 2.5 micrometers across, about 1/30 the width of a human hair.
And the way those droplets form -
with scarce or plentiful
aerosol particles - could have serious implications for weather and climate change.
Black carbon
aerosols —
particles of carbon that rise into the atmosphere when biomass, agricultural waste, and fossil fuels are burned in an incomplete way — are important for understanding climate change, as they absorb sunlight, leading to higher atmospheric temperatures, and can also coat Arctic snow
with a darker layer, reducing its reflectivity and leading to increased melting.
Until recently, the U.S. Department of Homeland Security has been investigating whether seeding storm clouds
with pollution - size
aerosols (
particles suspended in gas) might help slow tropical cyclones.
Albedo modification would work by lacing the atmosphere
with tiny
particles or
aerosols that would reflect sunlight and mimic natural processes.
Ginot and his team of researchers can also track
aerosols — small
particles in the atmosphere that fall
with snow and get trapped and stored in the ice, layer by layer, as the years pass.
Preliminary analyses show that most of the pollution was sulphate
aerosols — along
with dust and carbonaceous
particles such as black carbon.
Aerosol pollution also affects the formation of clouds, which are seeded
with dust
particles in the atmosphere.
Previous studies
with primates suggest that
aerosols of most biothreat agents, which are
particles dispersed in the air, are infectious.
Mikhailov, E., Vlasenko, S., Martin, S.T., Koop, T., and Pöschl, U.: Amorphous and crystalline
aerosol particles interacting
with water vapour: conceptual framework and experimental evidence for restructuring, phase transitions and kinetic limitations, Atmospheric Chemistry and Physics, 9, 9491 - 9522, 2009.
There are several variations on the so - called solar geoengineering theme, but they all have the same end - goal: using
aerosols to blanket our atmosphere
with reflective
particles in order to quickly lower global temperatures.
Additionally, stimulated bacterial degradation might heavily affect the organic composition of nascent sea - spray
particles, upon which relies the ability of marine
aerosols to interact
with the climate system.
Getting the data used in these 30 - plus papers,
with more to come, required extensive coincident measurements of meteorology, sunlight comings and goings, trace gases, and
aerosol particles.
This research is the first to connect a commercial CCN,
with a CVI and mass spectrometers to study the chemistry of
aerosol particles that activate to cloud droplets.
In general, the risk of
aerosol transmission increases
with proximity and duration of exposure to the source; however, once aerosolized, certain pathogens may remain infective over long distances, depending on
particle size, the nature of the pathogen, and such environmental factors as temperature and humidity.3
Maybe one could add instead: «This downward radiation from greenhouse gases (and some fine solid air
particles («
aerosols») e.g. can be measured at the surface in nights
with clear sky and no other radiation sources in the atmosphere (e.g. Philipona and Dürr 2004 doi / 10.1029 / 2004GL020937).
A paper discussing the difficulty of getting from nm sized nucleation mode to a size that can generate cloud
particles is: Erupe, M. E., et al. (2010), Correlation of
aerosol nucleation rate
with sulfuric acid and ammonia in Kent, Ohio: An atmospheric observation, J. Geophys.
We also know quite accurately the spectral absorption characteristics for the absorbing gases, and how cloud and
aerosol particles interact
with thermal radiation.
It is shown that such photopolarimetric data are highly sensitive to the size distribution and refractive index of
aerosol particles, which reduces the nonuniqueness in
aerosol retrievals using such data as compared
with less comprehensive datasets.
I write it off as a very real effect that is not well characterized by the models, probably because these models don't model
with enough accuracy the effect of the additional
aerosol particles on cloud production to properly account for it's full effect on temperature.
The parameterization of the interactions are at all levels; from estimation of the geometric characterization of the
aerosols, to the numbers of
particles, to connections
with several important aspects of clouds, and finally to the interactions
with radiative energy transport.
Ambient submicron
particle measurements were made
with a high - resolution time - of - flight
aerosol mass spectrometer (AMS) at the north campus of the University of California Irvine, which is located in the SoCAB approximately 5 miles inland from the Pacific Ocean.
The remainder is made up
with the other minor greenhouse gases, ozone and methane for instance, and a small amount from
particles in the air (dust and other «
aerosols»).
It then combines
with pollutants from combustion — mainly nitrogen oxides and sulfates from vehicles, power plants and industrial processes — to create tiny solid
particles, or
aerosols, no more than 2.5 micrometers across, about 1/30 the width of a human hair.
Coupling these new measurements
with detailed cloud simulations that resolve the size distributions of
aerosols and cloud
particles, we found several lines of evidence indicating that most anvil crystals form on mid-tropospheric rather than boundary - layer
aerosols.
It is found that
with a number concentration of
aerosol particles of ∼ 102 — 103 cm − 3 (which corresponds to the
aerosol density in the deposited layer of about 1 — 10 mg / m2
with the layer thickness along the ray path of about 100 m) the solar radiation attenuation
with artificial
aerosol layers accounts for 1 to 10 %.
Associated
with human greenhouse gas production is the release of fine
particle known as
aerosols which have a temporary cooling effect (they last in the atmosphere less than a week).
This method uses consistency between direct normal and diffuse horizontal measurements together
with a special regression technique for retrieval of daily time series of column mean
aerosol particle size,
aerosol optical depth, NO2, ozone and water vapor column amounts together
with the instrument's calibration constants.
The position statement opens
with the following: «Careful and comprehensive scientific assessments have clearly demonstrated that the Earth's climate system is changing rapidly in response to growing atmospheric burdens of greenhouse gases and absorbing
aerosol particles (IPCC, 2007).
The cloud condensation nuclei counter measures the concentration of
aerosol particles by drawing an air sample through a column
with thermodynamically unstable supersaturated water vapor that can condense onto
aerosol particles.
Aerosols A suspension of airborne solid or liquid
particles,
with a typical size between a few nanometres and 10 μm that reside in the atmosphere for at least several hours.
This system measures
aerosol optical properties to better understand how
particles interact
with solar radiation and influence the Earth's radiation balance.
While these
particles soon fall back down to Earth and allow the planet to heat up again, the thinking
with so - called solar geoengineering is that this thin layer of reflective sulfate
aerosols would be replenished to help keep it cool.
With regard to the actual content of the press release quoted, it isn't clear if the process they report on (
aerosol particles, particularly organic chemicals, getting smaller over time) makes them better or worse at forming clouds and their other atmosphere cooling functions.
Cloud condensation nuclei:
Aerosol particles that provide a platform for the condensation of water vapor, resulting in clouds
with higher droplet concentrations and increased albedo.
Here, gasses react
with water to form
aerosol particles that linger in the stratosphere for one or two years, reflecting sunlight and heat from the sun, and cooling the planet.
However, there have been proposals to mitigate climate change not by decreasing greenhouse gas emissions, but by increasing the reflection of incoming solar radiation
with mirrors,
aerosols (small
particles), or other means.
It has been hypothesized that galactic cosmic rays (GCR) create atmospheric ions which facilitates
aerosol nucleation and new
particle formation
with a further impact on the cloud formation (Kazil et al., 2012; Pierce and Adams, 2009).
The AOS measures
aerosol optical properties to better understand how
particles interact
with solar radiation and influence the earth's radiation balance.
Aerosols - A collection of airborne solid or liquid
particles,
with a typical size between 0.01 and 10 micrometer (~ 0.00000039 and ~ 0.00039 inch) that reside in the atmosphere for at least several hours.
«Earth system models» include all that and much more: forests that can shrink or spread as conditions change; marine food webs that react as the oceans grow more acidic
with carbon dioxide; and
aerosol particles in the atmosphere that interact
with greenhouse gases, enhancing or sapping their warming power.
Recently it was suggested that the formation of new atmospheric
aerosol particles is connected
with the existence of thermodynamically stable 1 - to 2 - nm clusters, formed in the atmosphere by some nucleation mechanism.
Interactions
with the hydrological cycle, and additional impacts on the radiation budget, occur through the role of
aerosols in cloud microphysical processes, as
aerosol particles act as cloud condensation nuclei (CCN) and ice nuclei (IN).