Song and fellow researchers published research in 2007 that addressed assumptions in the ability of diesel exhaust organic aerosols to mix
with organic aerosols from tree evaporate.
Forest fires in the lower latitudes, however, are actually beneficial sources of black carbon because it is coupled
with organic aerosols and ends up reflecting light and heat, causing the surrounding area to cool.
Not exact matches
The cooling effect of
aerosols can partly offset global warming on a short - term basis, but many are made of
organic material that comes from sources that scientists don't fully understand, said Joost de Gouw, a research physicist at NOAA's Earth System Research Laboratory in Boulder, Colo., who is unaffiliated
with the studies.
With 18 different scenarios tested, the team calculated a range of peak formation of secondary organic aerosols when typical concentrations of limonene were introduced to ozone - rich environments with a range of air exchange ra
With 18 different scenarios tested, the team calculated a range of peak formation of secondary
organic aerosols when typical concentrations of limonene were introduced to ozone - rich environments
with a range of air exchange ra
with a range of air exchange rates.
However, to make climate models more accurate, we are focused on developing a better understanding of the dynamics of
organic aerosols formed from plant - based
organic vapors and their interaction
with aerosols emitted from human activities,» said Dr. Chen Song, a PNNL atmospheric scientist.
The PNNL study measured how, in the atmosphere, these
aerosols interact
with and mix
with other volatile or semi-volatile
organic compounds, the carbon - centric chemicals that evaporate from both natural and human - made sources.
Additionally, stimulated bacterial degradation might heavily affect the
organic composition of nascent sea - spray particles, upon which relies the ability of marine
aerosols to interact
with the climate system.
Analyses of the ground and aircraft data performed by Setyan et al. (2012), Shilling et al. (2013), and Kleinman et al. (2016) showed that
organic aerosol production increased when human - caused emissions from Sacramento mixed
with air rich in isoprene, an
organic compound wafting from many plants that originate in the area's foothills.
How do
organic aerosols from biomass burning, which you can see in the red dots, intersect
with clouds and rainfall patterns?
All variables» short names that contained «pom» (total particulate
organic matter
aerosol) were changed to «oa» versions (total particulate
organic matter
aerosol) to conform to the CMIP5 tables, and to avoid confusion
with «poa» (primary particulate
organic matter
aerosol).
With regard to the actual content of the press release quoted, it isn't clear if the process they report on (
aerosol particles, particularly
organic chemicals, getting smaller over time) makes them better or worse at forming clouds and their other atmosphere cooling functions.
Cointegration indicates that internal climate variability and / or the omission of some components of radiative forcing (e.g., stratospheric water vapor, black or
organic carbon, nitrite
aerosols, etc.) do not impart a stochastic or deterministic trend that would interfere
with the interpretation of temperature changes at the subdecadal scale (SI Appendix).
The response of biogenic secondary
organic carbon
aerosol production to a temperature change, however, could be considerably lower than the response of biogenic VOC emissions since
aerosol yields can decrease
with increasing temperature.
The data generated in this laboratory is used to reduce the uncertainty associated
with representing the
organic aerosol lifecycle in climate models.
All secondary
aerosols (sulphuric, nitrates and
organics) are computed on - line together
with the
aerosol associated water.
The present 3 - D modeling study focuses on
aerosol chemical composition change since preindustrial times considering the secondary
organic aerosol formation together
with all other main
aerosol components including nitrate.
The climate feedbacks involved
with these changes, which are key in understanding the climate system as a whole, include: + the importance of
aerosol absorption on climate + the impact of
aerosol deposition which affects biology and, hence, emissions of
aerosols and
aerosol precursors via
organic nitrogen,
organic phosphorus and iron fertilization + the importance of land use and land use changes on natural and anthropogenic
aerosol sources + the SOA sources and impact on climate,
with special attention on the impact human activities have on natural SOA formation In order to quantitatively answer such questions I perform simulations of the past, present and future atmospheres, and make comparisons
with measurements and remote sensing data, all of which help understand, evaluate and improve the model's parameterizations and performance, and our understanding of the Earth system.
In particular, we evaluate non-sea-salt sulfate (nss - SO4 =), ammonium (NH4 +), nitrate (NO3 --RRB-, black carbon (BC), sea - salt, dust, primary and secondary
organics (POA and SOA)
with a focus on the importance of secondary
organic aerosols.
Topics that I work on or plan to work in the future include studies of: + missing
aerosol species and sources, such as the primary oceanic
aerosols and their importance on the remote marine atmosphere, the in - cloud and
aerosol water aqueous formation of
organic aerosols that can lead to brown carbon formation, the primary terrestrial biological particles, and the
organic nitrogen + missing
aerosol parameterizations, such as the effect of
aerosol mixing on cloud condensation nuclei and
aerosol absorption, the semi-volatility of primary
organic aerosols, the importance of in - canopy processes on natural terrestrial
aerosol and
aerosol precursor sources, and the mineral dust iron solubility and bioavailability + the change of
aerosol burden and its spatiotemporal distribution, especially
with regard to its role and importance on gas - phase chemistry via photolysis rates changes and heterogeneous reactions in the atmosphere, as well as their effect on key gas - phase species like ozone + the physical and optical properties of
aerosols, which affect
aerosol transport, lifetime, and light scattering and absorption,
with the latter being very sensitive to the vertical distribution of absorbing
aerosols +
aerosol - cloud interactions, which include cloud activation, the
aerosol indirect effect and the impact of clouds on
aerosol removal + changes on climate and feedbacks related
with all these topics In order to understand the climate system as a whole, improve the
aerosol representation in the GISS ModelE2 and contribute to future IPCC climate change assessments and CMIP activities, I am also interested in understanding the importance of natural and anthropogenic
aerosol changes in the atmosphere on the terrestrial biosphere, the ocean and climate.
Theoretically, coatings of essentially non-absorbing components such as
organic carbon or sulphate on strongly absorbing core components such as black carbon can increase the absorption of the composite
aerosol (e.g., Fuller et al., 1999; Jacobson, 2001a; Stier et al., 2006a),
with results backed up by laboratory studies (e.g., Schnaiter et al., 2003).
However, sulphate is invariably internally and externally mixed to varying degrees
with other compounds such as biomass burning
aerosol (e.g., Formenti et al., 2003), fossil fuel black carbon (e.g., Russell and Heintzenberg, 2000),
organic carbon (Novakov et al., 1997; Brock et al., 2004), mineral dust (e.g., Huebert et al., 2003) and nitrate
aerosol (e.g., Schaap et al., 2004).